For what it's worth, I ended up putting Marginalia Search behind Cloudflare to deal with what I assume is the same group. At worst I saw 30k queries per hour.
My unsubstantiated hunch based on looking at the types of queries, which at least for me were over-specified as all hell and within the sphere of pharmaceuticals, e-shopping and the like, is that they're gambling on the search engine being backed by Google or Bing, and they're effectively trying to poison their typeahead suggestion data.
I'd guess they're just aiming their gatling gun at whatever sites has an opensearch specification without much oversight.
It's also crossed my mind it might be some sketchy law firm looking for DMCA violations, since a fair bunch of the queries looked like they were after various forms of contraband. Seems weird they'd use a botnet though. Like most of the IPs seemed to be like enterprise routers with public facing admin pages and the like. Does not seem above board at all.